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Changes in magmatism and sedimentation along the late Neoproterozoic-early Paleozoic Ross orogenic belt in Antarctica have been linked to the cessation of convergence along the Mozambique belt during the assembly of East-West Gondwana. However, these interpretations are non-unique and are based, in part, on limited thermochronological data sets spread out along large sectors of the East Antarctic margin. We report new 40Ar/39Ar hornblende, muscovite, and biotite age data for plutonic (n = 13) and metasedimentary (n = 3) samples from the Shackleton–Liv Glacier sector of the Queen Maud Mountains in Antarctica. Cumulative 40Ar/39Ar age data show polymodal age peaks (510 Ma, 491 Ma, 475 Ma) that lag peaks in U-Pb igneous crystallization ages, suggesting igneous and metamorphic cooling following magmatism within the region. The 40Ar/39Ar ages are similar to ages in other sectors of the Ross orogen, but younger than detrital mineral 40Ar/39Ar cooling ages indicative of older magmatism and cooling of unexposed inboard areas along the margin. Detrital zircon trace element abundances suggest that the widespread onset of magmatism in outboard localities of the orogen correlates with a ~560–530 Ma decrease in crustal thickness. The timing of crustal thinning recorded by zircon in magmas overlaps with other evidence for the timing of crustal extension, suggesting that the regional onset of magmatism with subsequent igneous and metamorphic cooling probably reflects slab rollback that coincided with possible global plate motion changes induced during the final assembly of Gondwana. 

Orogenic crustal thickening leads to increased continental elevation and runoff into the oceans, but there are fundamental uncertainties in the temporal patterns of thickening through Earth history. U‐Pb age and trace element data in detrital zircons from Antarctica are consistent with recent global analyses suggesting two dominant peaks in average crustal thickness from ~2.6 to 2.0 Ga and ~0.8 to 0.5 Ga. Shifts in marine carbonate 87Sr/86Sr ratios show two primary peaks that post‐date these crustal thickness peaks, suggesting significant weathering and erosion of global continental relief. Both episodes correlate well with zircon trace element and isotope proxies indicating enhanced crustal and fluid input into subduction zone magmas. Increased crustal thickness correlates with increased passive margin abundance and overlaps with snowball Earth glaciations and atmospheric oxygenation, suggesting a causal link between continental rift‐drift phases and major transitions in Earth's atmospheric and oceanic evolution. 

Very large eruptions (>50 km 3 ) and supereruptions (>450 km 3 ) reveal Earth’s capacity to produce and store enormous quantities (>1000 km 3 ) of crystal-poor, eruptible magma in the shallow crust. We explore the interplay between crustal evolution and volcanism during a volcanic flare-up in the Taupo Volcanic Zone (TVZ, New Zealand) using a combination of quartz-feldspar-melt equilibration pressures and time scales of quartz crystallization. Over the course of the flare-up, crystallization depths became progressively shallower, showing the gradual conditioning of the crust. Yet, quartz crystallization times were invariably very short (<100 years), demonstrating that very large reservoirs of eruptible magma were transient crustal features. We conclude that the dynamic nature of the TVZ crust favored magma eruption over storage. Episodic tapping of eruptible magmas likely prevented a supereruption. Instead, multiple very large bodies of eruptible magma were assembled and erupted in decadal time scales.